The Natures
Natural SingLets keep the familiar letter names A, B, C, D, E, and G, while F shifts to Fi. In pronunciation, these correspond to /eɪ/, /bi/, /si/, /di/, /i/, /fi/, and /dʒi/.
Note F gets rid of its alphabetic pronunciation of /ɛf/, two discrete phones, and obtains /fi/, a CV.
This lets the natural domain preserve direct letter-name identity while improving singability where it is most needed.